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Composite Materials

 Composite Materials


After a first observation they were “re-discovered” at the beginning of the 90s and immediately started to cover a fundamental role in several scientific branches, from Physics to Chemistry, going through Medicine and Biology. In the Material Science and Engineering field a large number of studies have been conducted on carbon nanotubes, as a consequence of their extraordinary physical, technological and mechanical properties. For what concerns this research, they have been largely investigated as reinforcement materials in composites. Since 1991 a large number of attempts have been conducted, trying to exploit the outstanding potential of this carbonaceous material, in order to improve the properties of several matrices. The most important application is the production of polymer matrices composites (PMCs), but in last decades an increasing number of metal matrix ones (MMCs) have been presented and recently also ceramic matrix (CMCs) applications have been attempted. Despite massive efforts focused on CNTs-composites, the potential of employing this reinforcement materials has not yet been fully exploited. This lack is substantially due to the difficulties associated with the dispersion of entangled carbon nanotubes during processing and poor interfacial interaction between CNTs and matrix materials. The dispersion states of the nanotubes involve complicated phenomena, since the carbon nanotubes are produced in bundles or bundle aggregations. The states are affected by at least two competitive interactions: (1) the interactions of van der Waals forces, among carbon nanotube threads, and (2) the interactions between carbon nanotube threads and dispersion medium. The characteristics of single carbon nanotube and of bundles of carbon nanotubes are completely different. CNTs must be uniformly dispersed to the level of isolated tubes individually wetted by the matrix. This is necessary in order to achieve efficient load transfer to the reinforcement network. This also results in a more uniform stress distribution and minimises the presence of stress concentration centres. 

     Because of these reasons the very first aspect of this work has been the study of the dispersion state of nanotubes. The aim of the experiments was not only to obtain a good dispersion and distribution of the CNTs, but also to evaluate their dispersion grade. Indeed, due to their nanosize and to their carbonaceous nature, few simple experimental techniques result suitable for this purpose. In addition, the objective was also to use dispersion techniques which do not imply the utilisation of 7 high amount of solvents, reagents or surfactants, and so the aim was to develop a process as simple, low costs and as environmental friendly as possible.
The second part of the work consisted in the application of the carbon nanotubes to the production of new materials for technological applications, with improved mechanical properties. Three composite materials with different matrices have been designed, developed and produced: a polymer matrix composite, a ceramic matrix and a metal matrix one.
Also in these cases the aim of the work was the tuning of simple and possibly low costs production systems. 

      For PMCs a polyvinyl butyral matrix has been used and the composites were obtained by a deeply studied technique in the research group: the tape casting technology. The same approach was also used in the case of CMCs: tape casted silicon carbide matrix composites reinforced by carbon nanotubes have been produced. Finally a third matrix has been experimented: MMCs were investigated starting from pure aluminium powders. For Al matrix composites a particular technique was used: the sintering was obtained starting from a powder metallurgy approach and exploiting electric current and pressure (Electric Current Assisted Sintering approach).
For all the three different composite materials, after the development of the production route and the preparation of several specimens, a characterization step followed. The materials were characterized in terms of physical properties, morphology and microstructure, and mechanical behaviour.


    Composite materials are gaining wide spread acceptance, due to their characteristic behavior and high strength to weight ratio. Of these aluminium metal matrix composites are finding increased applications, because of their improved mechanical (such as hardness, young’s modulus, yield strength, and ultimate tensile strength due to the presence of micro-sized reinforcement particles into matrix material), physical and tribological properties and also the thermal conductivity of composite material are good. A metal matrix composite (MMCs) consists of a metallic alloy matrix (such as aluminium, magnesium, and titanium). Typically reinforced with a ceramic phase in the form of particles, platelets, whiskers, short fibers and continuously aligned fibers. Aluminium alloy reinforced with various particulate ceramics particles.
Fabrication of casting is done by stir casting processes among all the different processes.
Tungsten carbide is used as reinforcement material in aluminium alloy as matrix.

     Aluminium alloy are used in vast number of applications mostly used in automobile filed (such as engine cylinders, drive shafts, pistons, and brake rotors), industrial applications, aerospace applications and it is also useful in defence applications like torpedoes, manufacture of missile bodies, because of their low density, high strength to weight ratio, high thermal conductivity, high elastic modulus, and good structural rigidity. Aluminium alloy reinforced with various particulate ceramics particles are universally known as aluminium matrix composites (AMCs).
A composite may be defined as a structural material system that consists of two or more combined constituent’s material that are combined at a macroscopic level and are not soluble in each other. One constituent is called the reinforcing phase and the one in which it is embedded is called the matrix. The bulk material forms the continuous phase that is the matrix (e.g. metals, polymers, etc) while the other acts as the discontinuous phase that is the reinforcements (e.g. fibers, whiskers, particulates, etc). While the reinforcing material usually carries the major amount of load, the matrix enable the load transfer by holding them together. 

     Metal matrix composites (MMCs) are important class of material with non metallic reinforcement incorporated in metal matrices. Aluminium (Al) alloy matrices mainly 2024, 5052, 6061, and 7071 have been widely used as matrix materials
The present investigation has been focused on tungsten carbide (WC) particulate composite formation by utilization of low grade powdered graphite (Gr) by its dispersion into aluminium matrix by stir casting method. The objective is to form the reinforcing phase within the metallic matrix by reaction of graphite with aluminium in the metallic melt.
In this investigation aluminium 2024 (Al 2024) is the base material and reinforced with tungsten carbide (WC) and graphite (Gr) is used (Al 2024/WC-Graphite).
ASP Mech999

ASP Mech999

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